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ChemicalBook CAS DataBase List 4-Fluoro-1H-pyrazole
35277-02-2

4-Fluoro-1H-pyrazole synthesis

5synthesis methods
-

Yield:35277-02-2 77%

Reaction Conditions:

with hydrazine dihydrochloride in ethanol;water at 55; for 0.5 h;

Steps:

28.C Step C: 4-fluoro-1H-pyrazole (28-d)
Hydrazine dihydro chloride (4.48g, 0.043mol) was added to a solution of (Z)-3- (dimethylamino)-2-fluoroacrylaldehyde, 28-c, (5g, 0.043mol) in 100 mL of 40%>V/V solution of EtOH in water, then the mixture was heated at 55 °C for 30 minutes. The reaction was cooled to room temperature, basified to pH=9 with a saturated solution of NaHCC"3 and the aqueous layer was extracted with Et20. The organic layers were combined and dried with Na2SC"4, the solvent was removed to give 3.6 g of the titled product, 28-d, as a yellow oil (77%)

References:

MERCK SHARP & DOHME CORP.;ZHOU, Changyou;ZOU, Wuxin;HUA, Yuxia;DANG, Qun WO2013/40790, 2013, A1 Location in patent:Page/Page column 87; 88

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