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ChemicalBook CAS DataBase List (5-broMo-6-Methylpyridin-3-yl)Methanol
1174028-23-9

(5-broMo-6-Methylpyridin-3-yl)Methanol synthesis

3synthesis methods
5-Bromo-6-methyl-nicotinic acid methyl ester

1174028-22-8
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(5-broMo-6-Methylpyridin-3-yl)Methanol

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Yield:1174028-23-9 84%

Reaction Conditions:

Stage #1: methyl 5-bromo-6-methylnicotinatewith diisobutylaluminium hydride in dichloromethane;toluene at -78 - 20;Inert atmosphere;
Stage #2: with Potassium sodium tartrate in dichloromethane;water monomer;toluene;

Steps:

7.c

(c) (5-Bromo-6-methyl-3-pyridinyl)methanolTo a solution of methyl 5-bromo-6-methyl-3-pyridinecarboxylate (76 mg, 0.330 mmol) in DCM (1.5 ml), DIBAL-H (1.5 M solution in toluene, 0.661 ml, 0.991 mmol) was added dropwise at -78° C. under N2. The reaction mixture was allowed to warm to rt and stirred overnight. To this solution was added saturated, aqueous NaK-tartrate solution followed by DCM. The organic phase was separated, dried and concentrated to afford 56 mg of (5-bromo-6-methyl-3-pyridinyl)methanol (56 mg, 84%) pure enough to be used in the next step.1H-NMR (δ, ppm, CDCl3): 8.45 (s, 1H), 7.97 (s, 1H), 4.73 (s, 2H), 2.70 (s, 3H).

References:

US2009/306089,2009,A1 Location in patent:Page/Page column 29

78686-77-8 Synthesis
Methyl 5-bromo-6-chloropyridine-3-carboxylate

78686-77-8
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(5-broMo-6-Methylpyridin-3-yl)Methanol

1174028-23-9
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